Decoding decoherence
05 Oct 2020



Quantum information leaks away from a muon implanted in a fluoride crystal

Crystal structure of F-mu-F in calcium fluorite

​​The muon (black sphere) strongly coupled to two fluorine nuclei (dark blue spheres), and weakly coupled to next-nearest neighbour fluorine nuclei (cyan spheres), embedded inside the fluorite structure of CaF2.


A team from the Department of Physics at Oxford University has observed the decoherence process that occurs within quantum mechanical systems. Despite the many potential advantages of quantum computation, the integrity of any quantum mechanical system is vulnerable to interactions with its environment which cause any stored information to be slowly lost – decoherence.

The group has shown that an interesting realisation of decoherence occurs when a spin-polarised muon, an unstable radioactive particle, is implanted inside a crystal of an inorganic fluoride. The positively-charged muon nestles between two negatively-charged fluoride ions, pulling them towards itself, creating an interacting bound F-μ-F unit, with the spins of the muon and the two fluorine nuclei embodying a coherently evolving quantum system. Weak interactions between this 'system' and its 'environment' (all other fluoride ions in the crystal) decohere the quantum information stored in the muon, degrading it irreversibly. This process can be followed by watching the quantum interference oscillations in the muon spin polarisation as a function of time.

The experiments were performed using very intense beams of spin-polarised muons on the MuSR instrument. In their paper published in Physical Review Letters, John Wilkinson and Stephen Blundell describe how the degrading of quantum information can be understood by calculating the entropy in the entangled muon and fluorine spins, though an exact description is prevented by the size of the Hilbert space of the environment. Nevertheless, a method has been developed to describe the decohering effect of the environment in detail by renormalizing the coupling to the nearby shell of fluorine ions by a factor that includes the sum of the contributions of all nuclei in the crystal, providing excellent agreement with the new high-statistics experimental data.

Muon-fluorine systems have been known for some time and provide a rare example of a situation in which the location of a muon inside a crystal can be accurately determined, crucial for using the muon as a quantitative probe of the behaviour of materials. Recent work in Oxford and elsewhere has led to new computational techniques to tackle this problem and this new work opens up the possibility to provide a very detailed map of the local decohering system of nuclear spins in a range of different fluoride crystal architectures.

Information and decoherence in a muon-fluorine coupled system, J. M. Wilkinson and S. J. Blundell, Physical Review Letters 125, 087201 (2020) (Editors’ suggestion)​

This article was written for the University of Oxford Department of Physics, and originally appeared on their website​

Contact: de Laune, Rosie (STFC,RAL,ISIS)